To further investigate the reinforcement effects of high-strength geotextiles in high-fill steep slopes, model tests were conducted to compare high-strength geotextiles with other different geosynthetic materials including common geotextiles and geogrids. The results indicated that high-strength geotextile-reinforced steep slopes showed better performance in reducing slope body settlement, lateral displacement, and additional vertical stress compared with those reinforced with common geotextiles and geogrids. At the same time, the influence of different laying methods of high-strength geotextile on the stress and deformation characteristics of the slope body was studied. The results showed that changing the laying methods of high-strength geotextiles could enhance the safety and stability of high-fill loess steep slopes. Among the five different laying methods, the reinforced laying method of digging two grooves downwards and laying geotextiles (concave×2) can effectively reduce the crest settlement and additional vertical stress of the reinforced steep slopes. The research results can provide a reference for the engineering application of high-strength geotextile-reinforced steep slopes.